Discrete dynamics of nanoparticle channelling in suspended graphene.

نویسندگان

  • Tim J Booth
  • Filippo Pizzocchero
  • Henrik Andersen
  • Thomas W Hansen
  • Jakob B Wagner
  • Joerg R Jinschek
  • Rafal E Dunin-Borkowski
  • Ole Hansen
  • Peter Bøggild
چکیده

We have observed a previously undescribed stepwise oxidation of mono- and few layer suspended graphene by silver nanoparticles in situ at subnanometer scale in an environmental transmission electron microscope. Over the range of 600-850 K, we observe crystallographically oriented channelling with rates in the range 0.01-1 nm/s and calculate an activation energy of 0.557 ± 0.016 eV. We present a discrete statistical model for this process and discuss the implications for accurate nanoscale patterning of nanoscale systems.

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عنوان ژورنال:
  • Nano letters

دوره 11 7  شماره 

صفحات  -

تاریخ انتشار 2011